Chile

Why not?

Spanish

Top 10 Locations:

Santiago Capital of Chile
San Pedro de Atatcama Northern town in Chile - useful entry or exit point for tours to Salar de Uyuni.
Punta Arenas Its a looong way south!
San Pedro de Atacama On a border of atacama, idyllic oasis of tranquillity. Here U can end Uyuni trip and spend another few days exploring Val de la Luna, Val de la Muerte y nearby Lagunas.
Valparaiso So called Valpa. Colourful small houses on the hills, all by pacific.
National Transport
Long Distance Bus: 

http://www.turbus.cl
surprising but buses are actually cheaper in Chile then in Argentina, and very comfortable

Long Distance Train: 

no train network

Airlines: 
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